人才信息库
韩阿丽
性 别 最高学历 博士研究生
职 称 研究员 专家类别 硕士生导师
部 门 沈阳材料科学国家研究中心/先进炭材料研究部
通讯地址 辽宁省沈阳市沈河区文化路72号,中国科学院金属研究所,先进炭材料研究部
邮政编码 110016 电子邮件 alhan@imr.ac.cn
电 话 +86-24-23971846 传 真  
简历:

教育和工作经历

2021-至今,中国科学院金属研究所,研究员。

2019-2021, 清华大学,博士后。

2016-2019, 阿卜杜拉国王科技大学 (KAUST),博士后。

2011-2016, 中国科学技术大学,工学博士。

研究领域:

面向碳中和的电催化能量转换材料的制备与应用,如析氢反应(HER),氢氧化反应(HOR), 氧还原反应(ORR)等。

承担科研项目情况:

1)国家自然科学基金青年项目,30万元,项目负责人,2023-2025。

2)中国科学院引才计划择优支持,400万元,项目负责人,2023-2025。

3)辽宁省优秀青年科学项目,50万元,项目负责人,2022-2024。

重要科研成果

1)提出双外延生长新思路,实现单层高纯V单原子掺杂的1T-WS2高析氢活性

二维金属硫化物比表面积大,边缘S位点有析氢活性且晶相可调,是替代Pt基贵金属的理想析氢材料之一。然而高析氢活性的1T金属相硫化物难以直接合成。为此我们提出双外延限域生长直接获得金属相硫化物的新思路,实现了高纯单层金属相WS2的直接一步合成。One-step synthesis of single-site vanadium substitution in 1T-WS2 monolayers for enhanced hydrogen evolution catalysis. Nat. Commun. 2021, 12, 709.

2)提出邻近金属单原子界面电子结构调控,证实调控效应可提高氧还原活性

Fe-N4单原子材料具有成本低,氧还原活性好等优点,然而Fe-N4氧还原材料对含氧中间体吸脱附距离理想性能仍有差距。为此我们提出邻近异质单原子调控机制优化Fe-N4电子结构,从而实现高活性氧还原活性。An Adjacent Atomic Platinum Site Enables Single Atom Iron with High Oxygen Reduction Reaction Performance. Angew. Chem. Int. Ed. 2021, 60, 19262-19271.

3)提出多原子位点电子结构调控,实现高活性高稳定酸性氧还原活性

Fe-N4结构的单原子催化剂其本征活性相对Pt基贵金属较低且稳定性差,探索高效且能保持长期耐用性的铁基原子分散催化剂极具挑战性。为此我们设计一种全新的预限制策略,构建了相邻Co金属原子团簇与Fe-N4单原子共存的结构用于高性能的质子交换膜燃料电池。Construction of Co4 Atomic Clusters to Enable Fe-N4 Motifs with Highly Active and Durable Oxygen Reduction Performance. Angew. Chem. Int. Ed. 2023, e202303185.

社会任职:
获奖及荣誉:

2014. 中国科学院朱李月华奖学金。

2014. 博士研究生国家奖学金。

2016. 中国科学技术大学优秀毕业生。

2021. 清华大学化学系优秀博士后、创新博士后。

代表论著:

共发表40余篇SCI论文,其中共同第一/通讯作者论文20余篇,包括1篇Nat. Commun.、2篇Angew. Chem. Int. Ed., 1篇Nano Lett.、1篇ACS Nano等。

注:#代表同等贡献作者,*代表通讯作者

1.Ali Han#, Wenming Sun#, Xin Wan#, Dandan Cai#, Xijun Wang, Feng Li, Jianglan Shui, Dingsheng Wang. Construction of Co4 Atomic Clusters to Enable Fe-N4 Motifs with Highly Active and Durable Oxygen Reduction Performance. Angew. Chem. Int. Ed. 2023, e202303185.

2.Ali Han#, Xiaofeng Zhou#, Xijun Wang#, Sheng Liu, Qihua Xiong, Qinghua Zhang, Lin Gu, Zechao Zhuang, Wenjing Zhang, Fanxing Li, Dingsheng Wang*, Lain-Jong Li* and Yadong Li. One-Step Synthesis of Single-Site Vanadium Substitution in 1T-WS2 Monolayers for Enhanced Hydrogen Evolution Catalysis. Nat. Commun. 2021, 12, 709.

3.Ali Han#, Xijun Wang#, Kun Tang, Zedong Zhang, Chenliang Ye, Kejian Kong, Haibo Hu, Lirong Zheng, Peng Jiang, Changxin Zhao, Qiang Zhang, Dingsheng Wang* and Yadong Li. An Adjacent Atomic Platinum Site Enables Single‐Atom Iron with High Oxygen Reduction Reaction Performance. Angew. Chem. Int. Ed. 2021, 60, 19262-19271.

4.Ali Han, Zedong Zhang, Jiarui Yang, Dingsheng Wang* and Yadong Li*. Carbon-Supported Single-Atom Catalysts for Formic Acid Oxidation and Oxygen Reduction Reactions. Small, 2021, 2004500.

5.Ali Han, Zedong Zhang, Dingsheng Wang* and Yadong Li. Atomic Thickness Catalysts: Synthesis and Applications. Small Methods. 2020, 2000248.

6.Ali Han, Areej Aljarb, Sheng Liu, Peng Li, Chun Ma, Fei Xue, Sergei Lopatin, Chih-Wen Yang, Jing-Kai Huang, Yi Wan, Xixiang Zhang, Qihua Xiong, Kuo-Wei Huang, Vincent Tung*, Thomas Anthopoulos* and Lain-Jong Li*. Growth of 2H Stacked WSe2 Bilayers on Sapphire. Nanoscale Horiz., 2019, 4, 1434-1442.

7.Ali Han, Hanyu Zhang, Ruihan Yuan, Hengxing Ji and Pingwu Du*. Crystalline Copper Phosphide Nanosheets as an Efficient Janus Catalyst for Overall Water Splitting; ACS Appl. Mater. Interfaces. 2017, 9 (3), 2240-2248.

8.Ali Han, Huanlin Chen, Hanyu Zhang, Zijun Sun and Pingwu Du*. Ternary Metal Phosphide Nanosheets as a Highly Efficient Electrocatalyst for Water Reduction to Hydrogen Over a Wide pH Range From 0 to 14; J. Mater. Chem. A, 2016, 4, 10195-10202.

9.Ali Han, Huanlin Chen, Zijun Sun, Jun Xu and Pingwu Du*. High Catalytic Activity for Water Oxidation Based on Nanostructured Nickel Phosphide Precursors; Chem. Commun, 2015, 51, 11626-11629.

10.Ali Han, Song Jin, Huanlin Chen, Hengxing Ji, Zijun Sun and Pingwu Du*. A Robust Hydrogen Evolution Catalyst Based on Crystalline Nickel Phosphide Nanoflakes on Three-dimensional Graphene/nickel Foam: High Performance for Electrocatalytic Hydrogen Production from pH 0–14; J. Mater. Chem. A, 2015, 3, 1941-1946. 

11.Ali Han, Haotian Wu, Zijun Sun, Hongxing Jia, Zhiping Yan, Hao Ma, Xiang Liu and Pingwu Du*. Green Cobalt Oxide (CoOX) Film with Nanoribbon Structures Electrodeposited from the BF2-Annulated Cobaloxime Precursor for Efficient Water Oxidation; ACS Appl. Mater. Interfaces; 2014, 6, 10929-10934.

12.Ali Han, Pingwu Du* Zijun Sun, Haotian Wu, Hongxing Jia, Rui Zhang, Zhenning Liang, Rui Cao*, and Richard Eisenberg*. Reversible Mechanochromic Luminescence at Room Temperature in Cationic Platinum(II) Terpyridyl Complexes; Inorg. Chem., 2014, 53, 3338-3344.

13.Ali Han, Hongxing Jia, Hao Ma, Shifan Ye, Haotian Wu, Haitao Lei, Yongzhen Han, Rui Cao* and Pingwu Du*. Cobalt Porphyrin Electrode Films for Electrocatalytic Water Oxidation; Phys. Chem. Chem. Phys., 2014, 16, 11209-11217.

14.Ali Han, Pingwu Du*. Facile Deposition of Cobalt Oxide Based Electrocatalyst on Low-cost and Tin-free Electrode for Water Splitting; J. Energy Chem. 2014, 23, 179-184.

15.Ali Han, Haotian Wu, Zijun Sun, Hongxing Jia and Pingwu Du*. Facile Deposition of Nanostructured Cobalt Oxide Catalysts from Molecular Cobaloximes for Efficient Water Oxidation; Phys. Chem. Chem. Phys., 2013, 15, 12534-12538.

16.Ali Han, Pingwu Du*. Platinum-Cobalt Dinuclear Complex: Synthesis, Photophysical Properties and Visible Light-Drive Hydrogen Production from Water; Chinese. J. Inorg. Chem., 2013, 29, 1703-1709.

17.Jing Zhu#, Min Liao#, Chen Zhao#, Menngmeng Liu, Ali Han*, Chunna Zhu, Yujia Sun, Meng Zhao, Sheng Ye*, Haiqun Cao*. A comprehensive review on semiconductor-based photocatalysts toward the degradation of persistent pesticides.

18.Mengmeng Liu#, Chunyan Zhang#, Ali Han#, Ling Wang, Yujia Sun, Chunna Zhu, Rui Li & Sheng Ye*. Modulation of morphology and electronic structure on MoS2-based electrocatalysts for water splitting. Nano Res., 2022, 15, 6862-6887.

19.Peng Li#,*, Ali Han#, Chenhui Zhang, Xin He, Junwei Zhang, Long Cheng, Lain-Jong Li, Guoxing Miao* and Xixiang Zhang*. Mobility Fluctuation-Controlled Linear Positive Magnetoresistance in 2D Semiconductor Bi2O2Se Nano-plates. ACS Nano 2020, 14, 9, 11319-11326.

20.Zhaodong Chu#, Ali Han#, Chao Lei, Sergei Lopatin, Peng Li, David Wannlund, Di Wu, Kevin Herrera, Xixiang Zhang, Allan H. MacDonald, Xiaoqin Li, Lain-Jong Li and Keji Lai*. Energy-Resolved Photoconductivity Mapping in a Monolayer–Bilayer WSe2 Lateral Heterostructure. Nano Lett., 2018, 18 (11), 7200-7206.

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