1993.9-1997.6 学士,内蒙古大学,化学系
1997.9-2003.3 博士,中国科学院金属研究所
2003.4-2007.9 JSPS,博士后,日本东北大学
2007.9-2008.9 助理研究员,中国科学院金属研究所
2008.9-2014.9 副研究员,中国科学院金属研究所
2014.9-2018.9 项目研究员,中国科学院金属研究所
2018-9- 至今 研究员,中国科学院金属研究所
单壁碳纳米管(SWCNT)的可控制备与应用性能
1.发展了多种单一导电属性单壁碳纳米管可控制备方法。
提出了原位刻蚀—浮动催化剂化学气相沉积法,率先宏量可控制备出半导体性/金属性富集的SWCNT,被公认为是最有效的制备单一导电属性SWCNT的方法之一(J. Am. Chem. Soc. 2011, 133(14):5232;ACS Nano, 2013, 7:6831;ACS Nano, 2014, 8:7156);设计制备了钴-铼高熔点双金属催化剂,通过热力学控制实现均一直径碳纳米管稳定形核,通过动力学调控实现催化剂和金属性碳纳米管低的结合能、与低能量和碳源供给,最终实现金属性碳纳米管相对快速生长,获得窄直径分布的金属性碳纳米管(ACS Nano 2022, 6, 1:232–2409)。
图1.(a)钴-铼催化剂的透射电镜照片,内嵌图为其粒径分布。(b)催化剂成分能谱面扫。(c)窄直径分布高纯度金属性单壁碳纳米管典型透射电镜照片,内嵌图为其直径分布。(d)633 nm波长激光拉曼呼吸模。
2.揭示了限制单壁碳纳米管(SWCNT)柔性透明导电薄膜性能的瓶颈,建立了管束尺寸调控和管间接触电阻调控新方法,实现了高光电性能SWCNT柔性透明导电薄膜的高效制备。
通过对浮动催化剂化学气相沉积系统内碳管生长的热力学和动力学条件优化,实现了“碳焊”、单根SWCNT薄膜的控制制备。研究发现,该碳焊结构可使金属性和半导体性碳管间的肖特基接触转变为欧姆接触,显著降低接触电阻,从而获得了在90%透光率下面电阻仅为25Ω/□的透明导电薄膜,比已报道性能提高2倍以上,已优于柔性基底上的ITO(Sci. Advances 2018, 4, eaap9264,日本专利6845259)。
图2.(a-c)单根、“碳焊”结构SWCNT薄膜不同倾转角的TEM 照片;(d)有碳焊结构薄膜晶体管器件的SEM、AFM(插图)照片及器件输运性能(e);(f)基于碳焊结构的柔性碳管透明导电薄膜与文献中报道典型数据及柔性基底上ITO的光电性能对比图。
上述相关工作入选国家自然科学基金委资助成果;牛津大学科学家Cordelia Seal在Nano Today(IF=20.7)上发表了针对此工作的评论文章,称此项工作使碳纳米管在柔性电子及光电子器件应用优势更明显;文章同时引用美国佛罗里达大学著名的薄膜晶体管专家Andrew Rinzler教授及斯坦福纳米材料学专家崔屹教授的高度评价;中国科学基金杂志(Science Foundation in China)也对该工作进行了重点报道。
3.发展了多种功能基元序构新方法,在柔性碳纳米管薄膜上构筑了单原子团簇、异质结、取向纳米晶等功能基元,开拓了高性能SWCNT薄膜在能量存储与转换、柔性传感、异质结太阳能电池、光电探测等领域的应用,推动了SWCNT薄膜的性能提升与应用。
利用具有优异透明导电特性的SWCNT薄膜为透明电极和空穴传输层,开展了SWCNT/Si异质结太能电池的构建与性能研究(Nano Energy 2018, 50:521; Nano Energy 2020, 69: 104442; Adv. Func. Mater. 2021, 31(37):2104396; J. Mater. Chem. A 2022, 10(9): 4644);研制出多种碳纳米管复合电催化材料,设计、制备了多种柔性电催化剂一体化碳纳米管薄膜,组装、构建了高性能锌空电池及全固态柔性锌空电池等(Energ. Environ. Sci. 2016, 9:3079; NPG Asia Mater. 2018, 10:e461; Adv. Sci. 2019, 6:1802177; Appl. Catal. B 2020, 269:118823; Appl. Catal. B 2021, 294:120239)
1.Peng-Xiang Hou,Frontiers in Materials-Special issue “The Surface Chemistry of Carbon Materials: Design, Characterization, and Key Role in Surface Processes and Interactions”,Topic editor.
2.Peng-Xiang Hou,Molecules-Special issue “Carbon Nanomaterials: Synthesis and Application”, Guest Editor.
3.Progress in Materials Science、Advanced Functional Materials、Advanced Energy Materials、Energy Storage Materials、ACS Nano、Chemical Engineering Journal、Nanoscale、Scientific Report、Carbon、Applied Surface Science等国际知名杂志审稿人。
1.合作指导的多名研究生获得国家奖学金、中国科学院院长优秀奖、光华奖学金、师昌绪奖学金等奖项。
2.2018年被认定为沈阳市拔尖人才。
3.2014年获得沈阳材料科学国家(联合)实验室青年创新奖。
4.2012、2015年,Carbon期刊“Excellence in Review Award”奖。
5.2010年发表的第一作者论文“Purification of carbon nanotubes”入选ELSEVIER出版社“Top 50 Highly Cited Articles by Chinese Mainland Authors 2006?2010”。
1. PX Hou#, Feng Zhang#, Li-li Zhang, Chang Liu*, Hui-Ming Cheng*, Synthesis of carbon nanotubes by floating catalyst chemical vapor deposition and their applications, Advanced Functional Materials, 2022, 32, 2108541. (封面论文, IF=18.81)
2. X Li, F Zhang, LL Zhang, ZH Ji, YM Zhao, ZW Xu*, Y Wang, PX Hou*, M Tian, HB Zhao, S Jiang, LQ Ping, HM Cheng, C Liu*, Kinetics-controlled growth of metallic single-wall carbon nanotubes from CoRex nanoparticles, ACS Nano 2022, 16, 1, 232–2409. (IF=15.88)
3. XG Hu, QW Wei, YM Zhao, PX Hou*, WC Ren, C Liu*, HM Cheng, FeCl3-functionalized graphene oxide/single-wall carbon nanotube/silicon heterojunction solar cells with an efficiency of 17.5%, Journal of Materials Chemistry A, 2022, 10(9): 4644-4652. (IF=12.73)
4. J Zhang, XG Hu, H Li, KY Ji, BW Li, XP Liu, YR Xiang, PX Hou*, C Liu, ZH Wu, YL Shen, SD Stranks, SRP Silva*, HM Cheng*, W Zhang*, High-performance ITO-free perovskite solar cells enabled by single-walled carbon nanotube films, Advanced Functional Materials, 2021, 31, 2104396. (IF=18.81)
5. Y Meng, JC Li, SY Zhao, C Shi, XQ Li, LL Zhang, PX Hou*, C Liu*, HM Cheng, Fluorination-assisted preparation of self-supporting single-atom Fe-N-doped single-wall carbon nanotube film as bifunctional oxygen electrode for rechargeable Zn-Air batteries, Applied Catalysis B: Environmental, 2021, 294, 120239. (IF=19.5)
6. A Majeed, X Li, PX Hou*, H Tabassum, LL Zhang, C Liu*, HM Cheng, Monolayer carbon-encapsulated Mo-doped Ni nanoparticles anchored on single-wall carbon nanotube film for total water splitting, Applied Catalysis B: Environmental, 2020, 269: 118823. (IF=19.6)
7. XG Hu, PX Hou*, JB Wu, X Li, J Luan, C Liu*, G Liu, HM Cheng, High-efficiency and stable silicon heterojunction solar cells with lightly fluorinated single-wall carbon nanotube films, Nano Energy, 2020, 69: 104442. (IF=17.88)
8. A Majeed, PX Hou*, F Zhang, H Tabassum, X Li, GX Li, C Liu*, HM Cheng, A freestanding single-wall carbon nanotube film decorated with N-doped carbon-encapsulated Ni nanoparticles as a bifunctional electrocatalyst for overall water splitting , Advanced Science, 2019, 6(12): 1802177. (IF=16.8)
9. XG Hu, PX Hou*, F Zhang, C Liu*, G Liu, HM Cheng, Small-bundle single-wall carbon nanotubes for high-efficiency silicon heterojunction solar cells, Nano Energy, 2018, 50: 521. (IF=17.88)
10. JC Li, ZQ Yang, DM Tang, LL Zhang, PX Hou*, SY Zhao, C Liu*, M Cheng, GX Li, F Zhang, HM Cheng, N-doped carbon nanotubes containing a high concentration of single iron atoms for efficient oxygen reduction, NPG Asia Materials, 2018, 10:e461. (IF=10.48)
11. S Jiang#, PX Hou#, ML Chen, BW Wang, DM Sun, DM Tang, Q Jin, QX Guo, DD Zhang, JH Du, KP Tai, J Tan, EI Kauppinen, C Liu*, HM Cheng*, Ultrahigh-performance transparent conductive films of carbon-welded isolated single-wall carbon nanotubes, Science Advances, 2018, 4: eaap9264. (IF=14.14)
12. A Majeed, PX Hou*, S Jiang, JC Li, LQ Ping, GX Li, F Zhang, C Liu,* HM Cheng, Carbon-encapsulated NiO nanoparticle decorated single-walled carbon nanotube thin films for binderless flexible electrodes of supercapacitors, Journal of Materials Chemistry A, 2017, 5(47): 24813–24819. (IF=12.73)
13. JC Li, PX Hou*, C Liu*, Heteroatom-doped carbon nanotube and graphene-based electrocatalysts for oxygen reduction reaction, Small, 2017, 13(45): 1702002. (IF=13.28)
14. JC Li#, PX Hou#, SY Zhao, C Liu, DM Tang, M Cheng, F Zhang, HM Cheng, A 3D bi-functional porous N-doped carbon microtube sponge electrocatalyst for oxygen reduction and oxygen evolution reactions, Energy & Environmental Science, 2016, 9(10): 3079–3084. (IF=38.53)
15. F Zhang#, PX Hou#, C Liu, BW Wang, H Jiang, ML Chen, DM Sun, JC Li, HT Cong, EI. Kauppinen, HM Cheng, Growth of semiconducting single-wall carbon nanotubes with a narrow band-gap distribution, Nature Communications, 2016, 7: 11160. (IF=14.92)
学术活动(近期国际国内会议报告及任职等):
1. Hou PX, Liu C, Cheng HM, Synthesis of high-performance transparent conductive films and their applications. 3rd Global Webinar on Applied Science, Engineering and Technology, 2022.02.19-20, Keynote presentation.
2. Co-editors of “The Surface Chemistry of Carbon Materials: Design, Characterization, and Key Role in Surface Processes and Interactions” (collaboration with Frontiers in Materials )
近期获得专利:
1.侯鹏翔,蒋松,刘畅,成会明,炭素溶接構造の単層カ一ボンナノチュ一ブフレ キシブル透明導電性フィルムの調製方法,专利号:6845259,授权日:2021.03.01。
2.侯鹏翔,焦新宇,刘畅,成会明,高强度、高导电性单壁碳纳米管纤维的湿法纺丝制备方法,202011365820.2,授权日:2022.4.5。
3.侯鹏翔,刘畅,成会明,石超,孙东明,吴安萍,浮动催化剂化学气相沉积法制备多壁碳纳米管膜的装置,ZL202120212810.9,授权日:2021.10.22。
4.侯鹏翔,石超,刘畅,成会明,一种快速选择性填充纳米粒子至碳纳米管管腔内的方法,ZL201711130179.2,授权日:2020.11.13。
5.侯鹏翔,蒋松,刘畅,成会明,一种碳焊结构单壁碳纳米管柔性透明导电薄膜及制备方法,ZL201610459221.4,授权日:2019.3.29。